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However, in its raw form, GPS taxi data does not offer information on the purpose (or intended activity) of travel. In this context, to enhance the utility of taxi GPS data sets, we propose a two-layer framework to identify the related activities of each taxi trip automatically and estimate the return trips and successive activities after the trip, by using geographic point-of-interest (POI) data and a combination of spatio-temporal clustering, Bayesian inference and Monte Carlo simulation. Two million taxi trips in New York, the United States of America, and ten million taxi trips in Shenzhen, China, are used as inputs for the two-layer framework. To validate each layer of the framework, we collect 6,003 trip diaries in New York and 712 questionnaire surveys in Shenzhen. 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